2019-03-172019-03-172014-10-07http://repositorio.colciencias.gov.co/handle/11146/34071Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g., the sensitivity enhancement ascribed to 2D-FS. Although the isotropically averaged spectroscopic signals depend on the quantum yield parameter r of the doubly excited-exciton manifold, it is shown that the reconstruction of the dynamics is insensitive to this parameter. Applications 2015 AIP to foundational and applied problems, as well as further extensions, are discussed.pdf10 páginasenginfo:eu-repo/semantics/embargoedAccessArtículo científicoContiene 38 referencias bibliográficas. Véase el documento adjunto10.1063/1.4919954TermodinámicaModelos matemáticosMétodos de simulaciónDinámica de sistemasTeoría de campos (física)Propiedades termodinámicas